I do - about 90% of my stuff is all natural.
I alternate between LUSH's Soak and Float and Prairieland Herbs' Tea Tree and Peppermint Shampoo for my dandruff.
I condition with Africa's Best Hair Mayo or some Tresemme Conditioner (the mayo is partially natural, and Tresemme isn't).
Then I spritz my hair with Oyin's Frank Juice, and rub melted shea butter into my hair, then twist/ put in bantu knots to airdry.
The next day, I lightly oil my scalp with Hairveda's Vatika Frosting or Oyin's Burnt Sugar Pomade.
I use baking soda to clarify my scalp, and I use apple cider vinegar rinses after conditioning. I'm still looking for a very good moisturizing conditioner that's all natural.
My styling products are currently LUSH's Goth Juice and Oyin's Shine and Define. Together, both work wonders in keeping away flyaways.